Smoke and clouds above the Southeast Atlantic: upcoming field campaigns probe absorbing aerosol’s impact on climate

ArticleFrom July through October, smoke from biomass burning fires on the southern African sub-continent are transported westward through the free troposphere over one of the largest stratocumulus cloud decks on our planet. Biomass burning aerosol (smoke) absorbs shortwave radiation efficiently. This fundamental property implicates smoke within myriad small-scale processes with potential large-scale impacts on climate that are not yet well-understood. A coordinated, international team of scientists from the United States, United Kingdom, France, South Africa and Namibia will provide an unprecedented interrogation of this smoke-and-cloud regime from 2016 to 2018, using multiple aircraft and surface-based instrumentation suites to span much of the breadth of the southeast Atlantic

Stratocumulus Cloud-Top Height Estimates and Their Climatic Implications

A depth-dependent boundary layer lapse rate was empirically deduced from 156 radiosondes released during six month-long research cruises to the southeast Pacific sampling a variety of stratocumulus conditions. The lapse-rate dependence on boundary layer height is weak, decreasing from a best fit of 7.6 to 7.2 K km⁻¹ as the boundary layer deepens from 800 m to 2 km. Ship-based cloud-base heights up to 800 m correspond well to lifting condensation levels, indicating well-mixed conditions, with cloud bases >800 m often 200–600 m higher than the lifting condensation levels. The lapse rates were combined with Moderate Resolution Imaging Spectrometer 11-μm-derived cloud-top temperatures and satellite microwave-derived sea surface temperatures to estimate stratocumulus cloud-top heights. The October-mean cloud-top height structure of the southeast Pacific was then spatially and diurnally characterized. Coastal shoaling is apparent, but so is a significant along-coast cloud-top height gradient, with a pronounced elevation of the cloud-top heights above the Arica Bight at ~20°S. Diurnal cloud-top height variations (inferred from irregular 4-times-daily sampling) can locally reach 250 m in amplitude, and they can help to visualize offshore propagation of free-tropospheric vertical motions. A shallow boundary layer associated with the Chilean coastal jet expands to its north and west in the afternoon. Cloud-top heights above the Arica Bight region are depressed in the afternoon, which may mean that increased subsidence from sensible heating of the Andes dominates an afternoon increase in convergence/upward motion at the exit of the Chilean coastal jet. In the southeast Atlantic during October, the stratocumulus cloud-top heights are typically lower than those in the southeast Pacific. A coastal jet region can also be identified through its low cloud-top heights. Coastal shoaling of the South Atlantic stratocumulus region is mostly uniform with latitude, in keeping with the more linear Namibian/Angolan coastline. The southeast Atlantic shallow cloudy boundary layer extends farther offshore than in the southeast Pacific, particularly at 15°S

Observations of Stratocumulus Clouds and Their Effect on the Eastern Pacific Surface Heat Budget along 20°S

This is the publisher's version, also available electronically from http://journals.ametsoc.org/doi/abs/10.1175/JCLI-D-11-00618.1.Widespread stratocumulus clouds were observed on nine transects from seven research cruises to the southeastern tropical Pacific Ocean along 20°S, 75°–85°W in October–November of 2001–08. The nine transects sample a unique combination of synoptic and interannual variability affecting the clouds; their ensemble diagnoses longitude–vertical sections of the atmosphere, diurnal cycles of cloud properties and drizzle statistics, and the effect of stratocumulus clouds on surface radiation. Mean cloud fraction was 0.88, and 67% of 10-min overhead cloud fraction observations were overcast. Clouds cleared in the afternoon [1500 local time (LT)] to a minimum of fraction of 0.7. Precipitation radar found strong drizzle with reflectivity above 40 dBZ. Cloud-base (CB) heights rise with longitude from 1.0 km at 75°W to 1.2 km at 85°W in the mean, but the slope varies from cruise to cruise. CB–lifting condensation level (LCL) displacement, a measure of decoupling, increases westward. At night CB–LCL is 0–200 m and increases 400 m from dawn to 1600 LT, before collapsing in the evening. Despite zonal gradients in boundary layer and cloud vertical structure, surface radiation and cloud radiative forcing are relatively uniform in longitude. When present, clouds reduce solar radiation by 160 W m−2 and radiate 70 W m−2 more downward longwave radiation than clear skies. Coupled Model Intercomparison Project phase 3 (CMIP3) simulations of the climate of the twentieth century show 40 ± 20 W m−2 too little net cloud radiative cooling at the surface. Simulated clouds have correct radiative forcing when present, but models have ~50% too few clouds

A FIRE-ACE/SHEBA Case Study of Mixed-Phase Arctic Boundary Layer Clouds: Entrainment Rate Limitations on Rapid Primary Ice Nucleation Processes

Observations of long-lived mixed-phase Arctic boundary layer clouds on 7 May 1998 during the First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment (FIRE)Arctic Cloud Experiment (ACE)Surface Heat Budget of the Arctic Ocean (SHEBA) campaign provide a unique opportunity to test understanding of cloud ice formation. Under the microphysically simple conditions observed (apparently negligible ice aggregation, sublimation, and multiplication), the only expected source of new ice crystals is activation of heterogeneous ice nuclei (IN) and the only sink is sedimentation. Large-eddy simulations with size-resolved microphysics are initialized with IN number concentration N(sub IN) measured above cloud top, but details of IN activation behavior are unknown. If activated rapidly (in deposition, condensation, or immersion modes), as commonly assumed, IN are depleted from the well-mixed boundary layer within minutes. Quasi-equilibrium ice number concentration N(sub i) is then limited to a small fraction of overlying N(sub IN) that is determined by the cloud-top entrainment rate w(sub e) divided by the number-weighted ice fall speed at the surface v(sub f). Because w(sub c) 10 cm/s, N(sub i)/N(sub IN)<< 1. Such conditions may be common for this cloud type, which has implications for modeling IN diagnostically, interpreting measurements, and quantifying sensitivity to increasing N(sub IN) (when w(sub e)/v(sub f)< 1, entrainment rate limitations serve to buffer cloud system response). To reproduce observed ice crystal size distributions and cloud radar reflectivities with rapidly consumed IN in this case, the measured above-cloud N(sub IN) must be multiplied by approximately 30. However, results are sensitive to assumed ice crystal properties not constrained by measurements. In addition, simulations do not reproduce the pronounced mesoscale heterogeneity in radar reflectivity that is observed

African smoke particles act as cloud condensation nuclei in the wintertime tropical North Atlantic boundary layer over Barbados

The number concentration and properties of aerosol particles serving as cloud condensation nuclei (CCN) are important for understanding cloud properties, including in the tropical Atlantic marine boundary layer (MBL), where marine cumulus clouds reflect incoming solar radiation and obscure the low-albedo ocean surface. Studies linking aerosol source, composition, and water uptake properties in this region have been conducted primarily during the summertime dust transport season, despite the region receiving a variety of aerosol particle types throughout the year. In this study, we compare size-resolved aerosol chemical composition data to the hygroscopicity parameter κ derived from size-resolved CCN measurements made during the Elucidating the Role of Clouds–Circulation Coupling in Climate (EUREC4A) and Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign (ATOMIC) campaigns from January to February 2020. We observed unexpected periods of wintertime long-range transport of African smoke and dust to Barbados. During these periods, the accumulation-mode aerosol particle and CCN number concentrations as well as the proportions of dust and smoke particles increased, whereas the average κ slightly decreased (κ=0.46±0.10) from marine background conditions (κ=0.52±0.09) when the submicron particles were mostly composed of marine organics and sulfate. Size-resolved chemical analysis shows that smoke particles were the major contributor to the accumulation mode during long-range transport events, indicating that smoke is mainly responsible for the observed increase in CCN number concentrations. Earlier studies conducted at Barbados have mostly focused on the role of dust on CCN, but our results show that aerosol hygroscopicity and CCN number concentrations during wintertime long-range transport events over the tropical North Atlantic are also affected by African smoke. Our findings highlight the importance of African smoke for atmospheric processes and cloud formation over the Caribbean.</p

Cloud System Evolution in the Trades (CSET): Following the Evolution of Boundary Layer Cloud Systems with the NSFNCAR GV

The Cloud System Evolution in the Trades (CSET) study was designed to describe and explain the evolution of the boundary layer aerosol, cloud, and thermodynamic structures along trajectories within the North Pacific trade winds. The study centered on seven round trips of the National Science FoundationNational Center for Atmospheric Research (NSFNCAR) Gulfstream V (GV) between Sacramento, California, and Kona, Hawaii, between 7 July and 9 August 2015. The CSET observing strategy was to sample aerosol, cloud, and boundary layer properties upwind from the transition zone over the North Pacific and to resample these areas two days later. Global Forecast System forecast trajectories were used to plan the outbound flight to Hawaii with updated forecast trajectories setting the return flight plan two days later. Two key elements of the CSET observing system were the newly developed High-Performance Instrumented Airborne Platform for Environmental Research (HIAPER) Cloud Radar (HCR) and the high-spectral-resolution lidar (HSRL). Together they provided unprecedented characterizations of aerosol, cloud, and precipitation structures that were combined with in situ measurements of aerosol, cloud, precipitation, and turbulence properties. The cloud systems sampled included solid stratocumulus infused with smoke from Canadian wildfires, mesoscale cloudprecipitation complexes, and patches of shallow cumuli in very clean environments. Ultraclean layers observed frequently near the top of the boundary layer were often associated with shallow, optically thin, layered veil clouds. The extensive aerosol, cloud, drizzle, and boundary layer sampling made over open areas of the northeast Pacific along 2-day trajectories during CSET will be an invaluable resource for modeling studies of boundary layer cloud system evolution and its governing physical processes

Stratus 9/VOCALS ninth setting of the Stratus Ocean Reference Station & VOCALS Regional Experiment

The Ocean Reference Station at 20°S, 85°W under the stratus clouds west of northern Chile is being maintained to provide ongoing climate-quality records of surface meteorology; air-sea fluxes of heat, freshwater, and momentum; and of upper ocean temperature, salinity, and velocity variability. The Stratus Ocean Reference Station (ORS Stratus) is supported by the National Oceanic and Atmospheric Administration’s (NOAA) Climate Observation Program. It is recovered and redeployed annually, with cruises that have come between October and December. During the 2008 cruise on the NOAA ship Ronald H. Brown to the ORS Stratus site, the primary activities were recovery of the Stratus 8 WHOI surface mooring that had been deployed in October 2007, deployment of a new (Stratus 9) WHOI surface mooring at that site; in-situ calibration of the buoy meteorological sensors by comparison with instrumentation put on board by staff of the NOAA Earth System Research Laboratory (ESRL); and observations of the stratus clouds and lower atmosphere by NOAA ESRL. A buoy for the Pacific tsunami warning system was also serviced in collaboration with the Hydrographic and Oceanographic Service of the Chilean Navy (SHOA). The DART (Deep-Ocean Assessment and Reporting of Tsunami) carries IMET sensors and subsurface oceanographic instruments. A DART II buoy was deployed north of the STRATUS buoy, by personnel from the National Data Buoy Center (NDBC) Argo floats and drifters were launched, and CTD casts carried out during the cruise. The ORS Stratus buoys are equipped with two Improved Meteorological (IMET) systems, which provide surface wind speed and direction, air temperature, relative humidity, barometric pressure, incoming shortwave radiation, incoming longwave radiation, precipitation rate, and sea surface temperature. Additionally, the Stratus 8 buoy received a partial CO2 detector from the Pacific Marine Environmental Laboratory (PMEL). IMET data are made available in near real time using satellite telemetry. The mooring line carries instruments to measure ocean salinity, temperature, and currents. The ESRL instrumentation used during the 2008 cruise included cloud radar, radiosonde balloons, and sensors for mean and turbulent surface meteorology. Finally, the cruise hosted a teacher participating in NOAA’s Teacher at Sea Program.Funding was provided by the National Oceanic and Atmospheric Administration under Grant No. NA17RJ1223 for the Cooperative Institute for Climate and Ocean Research (CICOR)

Intercomparison of cloud model simulations of Arctic mixed‐phase boundary layer clouds observed during SHEBA/FIRE‐ACE

An intercomparison of six cloud‐resolving and large‐eddy simulation models is presented. This case study is based on observations of a persistent mixed‐phase boundary layer cloud gathered on 7 May, 1998 from the Surface Heat Budget of Arctic Ocean (SHEBA) and First ISCCP Regional Experiment ‐ Arctic Cloud Experiment (FIRE‐ACE). Ice nucleation is constrained in the simulations in a way that holds the ice crystal concentration approximately fixed, with two sets of sensitivity runs in addition to the baseline simulations utilizing different specified ice nucleus (IN) concentrations. All of the baseline and sensitivity simulations group into two distinct quasi‐steady states associated with either persistent mixed‐phase clouds or all‐ice clouds after the first few hours of integration, implying the existence of multiple states for this case. These two states are associated with distinctly different microphysical, thermodynamic, and radiative characteristics. Most but not all of the models produce a persistent mixed‐phase cloud qualitatively similar to observations using the baseline IN/crystal concentration, while small increases in the IN/crystal concentration generally lead to rapid glaciation and conversion to the all‐ice state. Budget analysis indicates that larger ice deposition rates associated with increased IN/crystal concentrations have a limited direct impact on dissipation of liquid in these simulations. However, the impact of increased ice deposition is greatly enhanced by several interaction pathways that lead to an increased surface precipitation flux, weaker cloud top radiative cooling and cloud dynamics, and reduced vertical mixing, promoting rapid glaciation of the mixed‐phase cloud for deposition rates in the cloud layer greater than about 1 − 2 × 10−5 g kg−1 s−1 for this case. These results indicate the critical importance of precipitation‐radiative‐dynamical interactions in simulating cloud phase, which have been neglected in previous fixed‐dynamical parcel studies of the cloud phase parameter space. Large sensitivity to the IN/crystal concentration also suggests the need for improved understanding of ice nucleation and its parameterization in models